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Title
Computational fluid dynamics analysis of CO2 absorption intensification in an hollow fiber membrane contactor using SiO2 and carbon nanotubes nanofluids
Type Article
Keywords
air pollution, carbon capture, carbon nanotube, membrane technology, nanoparticles
Abstract
A numerical parametric analysis of CO2 removal from the air using silica (SiO2) and carbon nanotube (CNT) nanofluids (NFs) in a gas–liquid hollow fiber membrane contactor in the non-wetted condition is investigated in this work. Diffusion in radial and axial directions is considered in the tube, the shell compartments, and the membrane regarding the convection mechanism. Different significant factors, including liquid and gas flow rates, membrane porosity, inlet concentration of CO2, liquid temperature, number of fibers, and nanoparticle diameters, are investigated in viable ranges. The finite element method is implemented to solve governing equations. The model output is validated against the experimental data of CO2 absorption with NFs, and an acceptable agreement is obtained. The results of the simulation indicate the CNT NFs outperform SiO2 NFs in CO2 absorption. Also, the performance of CO2 removal improves with the nanoparticle diameter reduction in the base fluid, inlet CO2 concentration, gas flow rate, and temperature. In the tube, by adding 0.5 wt % CNT and silica nanoparticles, the absorption rate improves by 47.6% and 39.6%, respectively. Finally, three correlations among significant parameters to predict CO2 removal is presented due to the lack of specific correlations for this model in the literature.
Researchers Fatemeh Keramat (Second researcher) , Ahmad Azari (Third researcher) , Shahriar Osfouri (Fourth researcher)